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Transition-metal dichalcogenides host a variety of charge-density-wave phases that couple lattice, charge, and correlation effects. In 1T -TaS2, the commensurate and nearly commensurate states are well characterized, yet the transition near 350 K into the incommensurate phase has lacked direct momentum-resolved insight. Here, we use temperature-dependent angle-resolved photoemission spectroscopy to track the electronic structure across this transition. We observe a suppression of quasiparticle spectral weight at the Brillouin-zone center, coincident with the transport anomaly, but without clear evidence of a full band-gap opening. The transition appears to involve momentum-dependent redistribution of spectral weight, consistent with a loss of coherence that reshapes the Fermi surface while leaving conduction dispersions largely intact. These results suggest that the nearly commensurate–incommensurate transition may not align with a conventional metal-insulator transition picture, but rather as an electronic reconstruction driven by loss of coherence. Our work provides new microscopic insight into the resistivity anomaly near room temperature and may guide design principles for collective electronic switching in transition-metal dichalcogenidesmore » « less
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Korshunov, A; Hu, H; Subires, D; Jiang, Y; Călugăru, D; Feng, X; Rajapitamahuni, A; Yi, C; Roychowdhury, S; Vergniory, M G; et al (, Nature Communications)Abstract Geometrically frustrated kagome lattices are raising as novel platforms to engineer correlated topological electron flat bands that are prominent to electronic instabilities. Here, we demonstrate a phonon softening at thekz = πplane in ScV6Sn6. The low energy longitudinal phonon collapses at ~98 K andq = $$\frac{1}{3}\frac{1}{3}\frac{1}{2}$$ due to the electron-phonon interaction, without the emergence of long-range charge order which sets in at a different propagation vectorqCDW = $$\frac{1}{3}\frac{1}{3}\frac{1}{3}$$ . Theoretical calculations corroborate the experimental finding to indicate that the leading instability is located at$$\frac{1}{3}\frac{1}{3}\frac{1}{2}$$ of a rather flat mode. We relate the phonon renormalization to the orbital-resolved susceptibility of the trigonal Sn atoms and explain the approximately flat phonon dispersion. Our data report the first example of the collapse of a kagome bosonic mode and promote the 166 compounds of kagomes as primary candidates to explore correlated flat phonon-topological flat electron physics.more » « less
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Rajapitamahuni, A.; Tao, L. L.; Hao, Y.; Song, J.; Xu, X.; Tsymbal, E. Y.; Hong, X. (, Physical Review Materials)
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